团队结构

赵 奎

教育与工作背景:

2015-至今  william威廉官网(教授、博士生导师)

2010-2015    博士后,沙特阿卜杜拉国王科技大学、美国斯坦福大学,合作导师:Prof. Aram Amassian, Prof. Michael McGehee

2004-2009    博士,中国科学经理春应用化学研究所,导师:韩艳春研究员

2000-2004    学士,吉林大学化学学院

Email:zhaok@snnu.edu.cn

课题组网站http://www.solarzhao.com/

科研背景:

聚焦新能源材料和器件研究(新型光伏技术 + 未来可穿戴柔性电子技术),发展交叉科学研究新手段与新技术,立足化学和物理深入认识物质形成规律,创新半导体材料基础理论,掌握半导体可控制备关键技术并推进应用验证。

主持项目:

维信诺公司光伏项目、中国辐射防护研究院项目、碑林环大学硬科技创新街区建设项目、三峡集团“揭榜挂帅”项目课题、XXX基础计划加强重点项目课题、中央高校重点支持项目、国家自然科学基金重点项目课题、国家自然科学基金面上项目、国家自然科学基金青年项目、陕西省重点研发计划项目、陕西省科技厅自然科学基金、科技部重点研发计划课题(参与)、中央高校重点支持项目、中央高校自由支持项目、中国科学院高分子物理国家重点实验室开放课题

成果和兼职:

获国家高层次人才、陕西省中青年科技创新领军人才、陕西九三学社碳中和研究院首席科学家、可再生能源和储能研究部部长、陕西省自然科学二等奖、陕西省高等学校科学技术研究优秀成果二等奖、西安市国际科技合作基地(负责人)、VEBLEO会士、中国科协科技青年论坛三等奖。担任InfoMatNano-Micro Lett.青年编委Frontier in ChemistryJournal of Modern Green Energy副主编Adv. Funct. Mater.Journal of Polymer Science等期刊客座编辑。撰写太阳电池团队标准1Adv. Energy Mater.等综述6篇书籍2个章节。课题组获得2023年陕西省优秀博士论文、第八届中国国际“互联网+”老员工创新创业大赛陕西省级银奖、第九届中国国际“互联网+”老员工创新创业大赛陕西省级银奖、第十一届“挑战杯”老员工创业计划竞赛陕西省铜奖。

课题组部分论文摘选:

1) Haojin Li,# Telun Li,# Chuang Ma,* Xinmei Liu, Lei Lang, Tinghuan Yang, Xin Song, Qingyue Cui, Zhou Yang, Shengzhong (Frank) Liu, Kui Zhao,* “One-Click Restart Recycling of Metal-Free Perovskite X-ray Detectors”, Adv. Mater. 2024, 2400783.

2) Chou Liu,# Tinghuan Yang,# Weilun Cai, Yajie Wang, Xin Chen, Shumei Wang, Wenliang Huang, Yachao Du, Nan Wu, Zhichao Wang, Yang Yang, Jiangshan Feng, Tianqi Niu, Zicheng Ding, Kui Zhao,* “Flexible indoor perovskite solar cells by in situ bottom-up crystallization modulation and interfacial passivation”, Adv. Mater. 2024, 2311562.

3) Huijing Liu, Jia Xu*, Huifang Han, Chenxu Zhao, Yao Fu, Kun Lang, Pengchen Zou, Xu Pan, Xinyu Gao,* Kui Zhao,* Jianxi Yao,* “Debridement Strategy by Pre-Bending Passivation for Flexible All-Inorganic Perovskite Solar Cells Beyond 70,000 Bending Cycles”, Adv. Funct. Mater. 2024, 2400975.

4) Yajie Wang,# Tinghuan Yang,# Weilun Cai, Peng Mao, Yang Yang, Nan Wu, Chou Liu, Shiqiang Wang, Yachao Du, Wenliang Huang, Guangtao Zhao, Zicheng Ding, Ningyi Yuan, Jianning Ding, Yufei Zhong,* Shengzhong (Frank) Liu, Kui Zhao,* “Defect Passivation Refinement in Perovskite Photovoltaics: Achieving Efficiency over 45% under Low-Light and Low-Temperature Dual Extreme Conditions”, Adv. Mater. 2024, 2312014.

5) Wenliang Huang, Zicheng Ding,* Zhongli Wang, Chenhui Xu, Ruipeng Li, Xinmei Liu, Shumei Wang, Yin Wu, Ru Qin, Yang Han, Yanhou Geng, Shengzhong (Frank) Liu, Yanchun Han,* Kui Zhao,* “Aligned Conjugated Polymer Nanofiber Networks in Elastomer Matrix for High-Performance Printed Stretchable Electronics”, Nano Lett. 2024, 24, 441.

6) Haojin Li,# Xinmei Liu,# Tinghuan Yang, Chuang Ma,* Yachao Du, Peng Xu, Lu Zhang, Xin Song, Qingyue Cui, Shengli Zhao, Zhou Yang, Shengzhong (Frank) Liu, Shengye Jin,* Kui Zhao,* “Flexible large-scale self-driven perovskite X-ray detector by precise heterogeneous integration”. ACS Energy Lett. 2024, 9, 64.

7) Yong Li,# Ting Nie,# Xiaodong Ren,* Yin Wu, Jing Zhang, Pengjun Zhao, Yuying Yao, Yucheng Liu, Jiangshan Feng, Kui Zhao,* Wenhua Zhang,* Shengzhong Liu,* “In situ formation of 2D perovskite seeding for record-efficiency indoor perovskite photovoltaic devices”, Adv. Mater. 2023, 2306870.

8) Yachao Du, Qingwen Tian,* Shiqiang Wang, Lei Yin, Chuang Ma, Zhiteng Wang, Lei Lang, Yingguo Yang, Kui Zhao,* Shengzhong (Frank) Liu*, “Crystallization Control Based on the Regulation of Solvent-Perovskite Coordination for High-Performance Ambient Printable FAPbI3 Perovskite Solar Cells”. Adv. Mater. 2023, 2307583.

9) Nan Wu,# Tinghuan Yang,# Zhichao Wang, Yin Wu, Yajie Wang, Chuang Ma, Haojin Li, Yachao Du, Di Zhao, Shuang Wang, Pengchi Liu, Wenliang Huang, Xiaodong Ren, Shengzhong (Frank) Liu, Kui Zhao*, “Stabilizing precursor solution and controlling crystallization kinetics simultaneously for high-performance perovskite solar cells”, Adv. Mater. 2023, 35, 2304809.

10) Shiqiang Wang,# Tinghuan Yang,# Yingguo Yang, Yachao Du, Wenliang Huang, Liwei Cheng, Haojin Li, Peijun Wang, Yajie Wang, Yi Zhang, Chuang Ma, Pengchi Liu, Guangtao Zhao, Zicheng Ding, Shengzhong (Frank) Liu, Kui Zhao,* “In situ self-elimination of defects via controlled perovskite crystallization dynamics for high-performance solar cells”, Adv. Mater. 2023, 35, 2305314.

11) Weilun Cai,# Tinghuan Yang,# Chou Liu, Yajie Wang, Shiqiang Wang, Yachao Du, Nan Wu, Wenliang Huang, Shumei Wang, Zhichao Wang, Xin Chen, Jiangshan Feng, Guangtao Zhao, Zicheng Ding, Xu Pan, Pengchen Zou, Jianxi Yao, Shengzhong (Frank) Liu, Kui Zhao,* “Interfacial Engineering for Efficient Low-Temperature Flexible Perovskite Solar Cells”, Angewandte Chemie, 2023, 62, e202309398.

12) Junwei Liu, Zhihua Zhou, Yuping Gao, Yin Wu, Jingjing Wang, Haojin Li, Qian Wang, Kangkang Zhou, Kaihu Xian, Yu Chen, Wenchao Zhao, Fei Zhang, Hang Yin, Yongsheng Liu*, Kui Zhao*, Jinyue Yan,* Long Ye,* “Polymer Synergy for Dopant-free and Efficient Hole Transport in Solar Cells and Photodetectors”, Energy Environ. Sci. 2023, D3EE02033A.

13) Lei Yin,# Wenliang Huang,# Junjie Fang,# Zicheng Ding,* Chengkai Jin, Yachao Du, Shumei Wang, Weilun Cai, Chou Liu, Guangtao Zhao, Yingguo Yang, Shengzhong (Frank) Liu, Tongle Bu,* and Kui Zhao,* “Crystallization control for ambient printed FA-based lead triiodide perovskite solar cells”, Adv. Mater. 2023, 35, 2303384.

14) Tinghuan Yang, Chuang Ma, Weilun Cai, Shiqiang Wang, Yin Wu, Jiangshan Feng,* Nan Wu, Haojin Li, Wenliang Huang, Zicheng Ding, Lili Gao, Shengzhong (Frank) Liu, Kui Zhao,* “Amidino-based Dion-Jacobson 2D perovskite for efficient and stable 2D/3D heterostructure perovskite solar cells”, Joule, 2023, 7, 574.

15) Tinghuan Yang,# Lili Gao,# Jing Lu, Chuang Ma, Yachao Du, Peijun Wang, Zicheng Ding, Shiqiang Wang, Peng Xu, Dongle Liu, Haojin Li, Xiaoming Chang, Junjie Fang, Wenming Tian,* Yingguo Yang, Shengzhong (Frank) Liu* Kui Zhao,* “One-stone-for-two-birds strategy to attain beyond 25% perovskite solar cells”, Nat. Commun., 2023, 14, 839.

16) Xin Song, Hagai Cohen, Jun Yin, Haojin Li, Jiayi Wang, Youyou Yuan, Renwu Huang, Qingyue Cui, Chuang Ma, Shengzhong (Frank) Liu, Gary Hodes,* Kui Zhao,* “Low Dimensional, Metal‐Free, Hydrazinium Halide Perovskite‐Related Single Crystals and Their Use as X‐Ray Detectors”, Small, 2023, 2300892.

17) Yachao Du, Qingwen Tian,* Shiqiang Wang, Tinghuan Yang, Lei Yin, Hao Zhang, Weilun Cai, Yin Wu, Wenliang Huang, Lu Zhang, Kui Zhao,* and Shengzhong (Frank) Liu*, “Manipulating the Formation of 2D/3D Heterostructure in Stable High-Performance Perovskite Solar Cells Based on Ambient-Printed CsPbI3”, Adv. Mater. 2022, 2, 2206451.

18) Shumei Wang, Wenliang Huang, Xinmei Liu, Shiqiang Wang, Haochen Ye, Shen Yu, Xin Song, Zhan Liu, Peijun Wang, Tinghuan Yang, Depeng Chu, Jing Gou, Mingjian Yuan, Lihua Chen, Baolian Su, Shengzhong (Frank) Liu, Kui Zhao,* “Ruddlesden–Popper Perovskite Nanocrystals Stabilized in Mesoporous Silica with Efficient Carrier Dynamics for Flexible X-Ray Scintillator”, Adv. Funct. Mater. 2022, 33, 2210765.

19) Jiayu Di, Haojin Li, Li Chen, Siyu Zhang, Yinhui Hu, Kai Sun, Bo Peng, Jie Su, Xue Zhao, Yuqi Fan, Zhenhua Lin, Yue Hao, Peng Gao, Kui Zhao,* Jingjing Chang,* “Low Trap Density Para-F Substituted 2D PEA2PbX4 (X = Cl, Br, I) Single Crystals with Tunable Optoelectrical Properties and High Sensitive X-Ray Detector Performance”, Research, 2022, 9768019.

20) Yin Wu, Zicheng Ding,* Qiang Zhang, Xiao Liang, Hanlin Hu, Hua Yang, Jianning Ding, Yanchun Han, Shengzhong (Frank) Liu, Kui Zhao,* “Increasing H-aggregates via sequential aggregation to enhance the hole mobility of printed conjugated polymer films”, Macromolecules, 2022, 55, 8609.

21) Chang-Feng Wang, Haojin Li, Qun Ji, Chuang Ma, Lang Liu, Heng-Yun Ye, Bo Cao, Guoliang Yuan, Hai-Feng Lu, Da-Wei Fu, Ming-Gang Ju,* Jinlan Wang, Kui Zhao,* Yi Zhang,* “Discovery of a 2D Hybrid Silver/Antimony‐Based Iodide Double Perovskite Photoferroelectric with Photostrictive Effect and Efficient X‐Ray Response”, Adv. Funct. Mater. 2022, 2205918.

22) Xinmei Liu,# Haojin Li,# Qingyue Cui, Shumei Wang, Chuang Ma, Nuo Bu, Tinghuan Yang, Xin Song, Yucheng Liu, Zhou Yang, Kui Zhao,* Shengzhong (Frank) Liu, “Molecular Doping of Flexible Lead‐Free Perovskite‐Polymer Thick Membranes for High‐Performance X‐Ray Detection”, Angew. Chem. Int. Ed., 2022, 61, 2209320.(Hot paper)

23) Qiuju Liu, Weilun Cai, Weiyan Wang, Haiqiao Wang, Yufei Zhong*, Kui Zhao,* “Controlling Phase Transition Towards Future Low-cost and Eco-friendly Printing Perovskite Solar Cells”, J. Phys. Chem. Lett. 2022, 21, 6503.

24) Chuang Ma, Haojin Li, Ming Chen, Yucheng Liu, Kui Zhao,* Shengzhong (Frank) Liu,* “Water-Resistant Lead-Free Perovskitoid Single Crystal for Efficient X-Ray Detection”, Adv. Funct. Mater. 2022, 32, 2202160.

25) Qingyue Cui, Nuo Bu, Xinmei Liu, Haojin Li, Zhuo Xu, Xin Song, Kui Zhao,* Shengzhong (Frank) Liu,* “Efficient Eco-friendly Flexible X-ray Detectors Based on Molecular Perovskite”, Nano Lett. 2022, 22, 5973.

26) Qingyue Cui, Shengzhong (Frank) Liu,* Kui Zhao,* “Structural and Functional Insights into Metal-Free Perovskites”, J. Phys. Chem. Lett. 2022, 13, 5168.

27) Chuang Ma, Lili Gao*, Zhuo Xu, Xiaotong Li, Xin Song, Yucheng Liu, Tinghuan Yang, Haojin Li, Yachao Du, Guangtao Zhao, Xinmei Liu, Mercouri G. Kanatzidis*, Shengzhong Frank Liu*, Kui Zhao*, “Centimeter-Sized 2D Perovskitoid Single Crystals for Efficient X-ray Photoresponsivity” Chem. Mater. 2022, 34, 4, 1699.

28) Zicheng Ding, Kui Zhao*, “Polymers for new energy technology” J. Polym. Sci. 2022, 60, 863–864.(As guest editor)

29) Yachao Du, Qingwen Tian*, Xiaoming Chang, Junjie Fang, Xiaojing Gu, Xilai He, Xiaodong Ren, Kui Zhao,* Shengzhong (Frank) Liu*, “Ionic Liquid Treatment for Highest-Efficiency Ambient Printed Stable All-Inorganic CsPbI3 Perovskite Solar Cells”, Adv. Mater. 2022, 34, 2106750.

30) Jing Lu, Tinghuan Yang, Tianqi Niu, Nuo Bu, Yalan Zhang, Shiqiang Wang, Junjie Fang, Xiaoming Chang, Tao Luo, Jialun Wen, Yingguo Yang, Zicheng Ding,* Kui Zhao,*, Shengzhong (Frank) Liu*, “Formamidinium-based Ruddlesden–Popper perovskite films fabricated via two-step sequential deposition: quantum well formation, physical properties and film-based solar cells”, Energy Environ. Sci., 2022, 15, 1144.

31) Dongle Liu, Zicheng Ding*, Yin Wu, Shengzhong Frank Liu, Yanchun Han, Kui Zhao*, “In Situ Study of Molecular Aggregation in Conjugated Polymer/Elastomer Blends toward Stretchable Electronics” Macromolecules 2022, 55, 1297.

32) Qingyue Cui,# Xin Song,# Yucheng Liu, Zhuo Xu, Haochen Ye, Zhou Yang, Kui Zhao,* Shengzhong (Frank) Liu,* “Halide-Modulated Self-Assembly of Metal-Free Perovskite Single Crystals for Bio-Friendly X-Ray Detection”, Matter, 2021, 4, 2490.

33) Kui Zhao*, G. N. Manjunatha Reddy,* Yanchun Han,* “Organic Semiconductors: Investigating the Processing-Structure-Property Relationships”, Front. Chem. 2021, 9:745170.(As Topic editor)

34) Xin Song, Qian Li, Jiang Han, Chuang Ma, Zhuo Xu, Haojin Li, Peijun Wang, Zhou Yang, Qingyue Cui, Lili Gao, Zewei Quan,* Shengzhong (Frank) Liu,* Kui Zhao*, “Highly Luminescent Metal‐Free Perovskite Single Crystal for Biocompatible X‐Ray Detector to Attain Highest Sensitivity”, Adv. Mater. 2021, 2102190.

35) Zicheng Ding, Kui Zhao,* Yanchun Han,* “Optimizing Morphology to Trade Off Charge Transport and Mechanical Properties of Stretchable Conjugated Polymer Films”, Macromolecules 2021, 54, 3907.

36) Kang Wang,† Changji Gao,† Zhuo Xu,† Qingwen Tian,* Xiaojing Gu, Lu Zhang, Shiang Zhang, Kui Zhao,* Shengzhong (Frank) Liu,* “In‐Situ Hot Oxygen Cleansing and Passivation for All‐Inorganic Perovskite Solar Cells Deposited in Ambient to Breakthrough 19% Efficiency”, Adv. Funct. Mater. 2021, 202101568.

37) Xilai He, Jiangzhao Chen, Xiaodong Ren,* Lu Zhang, Yucheng Liu, Jiangshan Feng, Junjie Fang, Kui Zhao,* Shengzhong (Frank) Liu,* “40.1% Record Low-Light-Solar-Cell-Efficiency by Holistic Trap-Passivation using Micron-Thick Perovskite Film”, Adv. Mater. 2021, 33, 2100770.

38) Xu Zhang, Tinghuan Yang, Xiaodong Ren, Lu Zhang, Kui Zhao,* Shengzhong (Frank) Liu,* “Film Formation Control for High Performance Dion–Jacobson 2D Perovskite Solar Cells”, Adv. Energy Mater. 2021, 11, 2002733.

39) Chuang Ma, Fang Chen, Xin Song, Ming Chen, Lili Gao, Peijun Wang, Jialun Wen, Zhou Yang, Youzhi Tang,* Kui Zhao,* Shengzhong (Frank) Liu* “Centimeter-Sized Molecular Perovskite Crystal for Efficient X-Ray Detection”, Adv. Funct. Mater. 2021, 2100691.

40) Xiaoming Chang, Yuanyuan Fan, Kui Zhao,* Junjie Fang, Dongle Liu, Ming-Chun Tang, Dounya Barrit, Detlef-M. Smilgies, Ruipeng Li, Jing Lu, Jianbo Li, Tinghuan Yang, Aram Amassian, Zicheng Ding, Yonghua Chen, Shengzhong (Frank) Liu*, Wei Huang,* “Perovskite Solar Cells towards Eco-friendly Printing”, Research, 2021, 16, 9671892. (ISSN: 2639-5274)

41) Chang-Feng Wang, Haojin Li, Mao-Guang Li, Yu Cui, Xin Song, Qin-Wen Wang, Jia-Ying Jiang, Miao-Miao Hua, Qi Xu, Kui Zhao,* Heng-Yun Ye,* Yi Zhang,* “Centimeter-Sized Single Crystals of Two-Dimensional Hybrid Iodide Double Perovskite (4,4-Difluoropiperidinium)4AgBiI8 for High-Temperature Ferroelectricity and Efficient X-Ray Detection”, Adv. Funct. Mater. 2021, 31, 2009457.

42) Xin Song, Gary Hodes,* Kui Zhao,* Shengzhong (Frank) Liu,* “Metal-Free Organic Halide Perovskite: A New Class for Next Optoelectronic Generation Devices”, Adv. Energy Mater. 2021, 2003331.

43) Xin Song, Qingyue Cui, Yucheng Liu, Zhuo Xu, Hagai Cohen, Chuang Ma, Yuanyuan Fan, Yunxia Zhang, Haochen Ye, Zhanhui Peng, Ruipeng Li, Yonghua Chen, Jianpu Wang, Huaming Sun, Zhou Yang, Zhike Liu, Zupei Yang, Wei Huang,* Gary Hodes,* Shengzhong (Frank) Liu,* Kui Zhao,* “Metal-free halide perovskite single crystals with very long charge lifetimes for efficient X-ray imaging”. Adv. Mater. 2020. 32, 2003353.

44) Guangbao Wu, Tinghuan Yang, Xing Li, Nafees Ahmad, Xuning Zhang, Shengli Yue, Jin Zhou,Yanxun Li, Hui Wang, Xinghua Shi, Shengzhong (Frank) Liu, Kui Zhao,* Huiqiong Zhou,* Yuan Zhang,* “Molecular Engineering for Two-Dimensional Perovskites with Photovoltaic Efficiency Exceeding 18%”, Matter, 2021, 4, 582.

45) Peijun Wang, Bolun Wang, Yucheng Liu, Lin Li, Hua Zhao, Yonghua Chen, Jiyang Li*, Shengzhong (Frank) Liu*, Kui Zhao,* “Ultrastable perovskite-zeolite composite enabled by encapsulation and in situ passivation”. Angew. Chem. Int. Ed. 2020, 59, 23100.

46) Xiaoming Chang, Junjie Fang, Yuanyuan Fan, Tao Luo, Hang Su, Yalan Zhang, Jing Lu, Leonidas Tsetseris, Thomas D. Anthopoulos,* Shengzhong (Frank) Liu,* Kui Zhao,* “Printable CsPbI3 perovskite solar cells with PCE of 19% via additive strategy”. Adv. Mater. 2020, 32, 2001243.

47) Yue Shen,# Yucheng Liu,# Haochen Ye, Yiting Zheng, Qi Wei, Yingdong Xia, Yonghua Chen,* Kui Zhao,* Wei Huang, Shengzhong (Frank) Liu,* “Centimeter-sized Single Crystal of Two-Dimensional Halide Perovskites Incorporating Straight Chain Symmetric Diammonium Ion for Efficient X-ray Detection”. Angew. Chem. Int. Ed. 2020, 59, 2-9.

48) Dounya Barrit,# Peirui Cheng,# Ming-Chun Tang, Detlef-M. Smilgies, Shengzhong (Frank) Liu, Thomas D. Anthopoulos,* Kui Zhao,* Aram Amassian,* “Room-Temperature Formation of α-FAPbI3 Perovskite Phase via PbI2 Solvation Enables High-Performance Solar Cells”. Adv. Funct. Mater. 2020, 1907442.

49) Jiangang Liu,* Ergang Wang,* Kui Zhao,* “Polymer Solar Cells: Molecular Design and Microstructure Control”. Front. Chem. 2020, DOI: 10.3389/fchem.2020.00697. (As Topic editor)

50) Kui Zhao,* Zhou Yang,* Shengzhong (Frank) Liu,* “Emerging Photovoltaic Materials and Devices”. Adv. Funct. Mater. 2019, 29, 1904014. (As Guest editor)

51) Tianqi Niu,# Jing Lu,# Xuguang Jia, Zhuo Xu, Ming-Chun Tang, Dounya Barrit, Ningyi Yuan, Jianning Ding, Xu Zhang, Yuanyuan Fan, Tao Luo, Yalan Zhang, Detlef-M. Smilgies, Zhike Liu, Aram Amassian, Shengye Jin, Kui Zhao,* “Interfacial engineering at the 2D/3D heterojunction for high-performance perovskite solar cells”. Nano Lett. 2019, 19, 7181.

52) Tao Luo,# Yalan Zhang,# Zhuo Xu, Tianqi Niu, Jialun Wen, Jing Lu, Shengye Jin, Shengzhong (Frank) Liu,* Kui Zhao,* “Compositional Control in Two-Dimensional Perovskites with Alternating Cations in the Interlayer Space for Photovoltaics with Efficiency over 18%”. Adv. Mater. 2019, 31, 1903848.

53) Guangbao Wu, Xing Li, Jiyu Zhou, Jianqi Zhang, Xuning Zhang, Xuanye Leng, Peijun Wang, Ming Chen, Dongyang Zhang, Kui Zhao,* Shengzhong (Frank) Liu, Huiqiong Zhou,* Yuan Zhang,* “Fine Multi-Phase Alignments in 2D Perovskite Solar Cells with Efficiency over 17% via Slow Post-Annealing”. Adv. Mater. 2019, 1903889.

54) Yuanyuan Fan, Junjie Fang, Xiaoming Chang, Ming-Chun Tang, Dounya Barrit, Zhuo Xu, Zhiwu Jiang, Jialun Wen, Huan Zhao, Tianqi Niu, Detlef-M. Smilgies, Shengye Jin, Zhike Liu, Er Qiang Li, Aram Amassian,* Shengzhong (Frank) Liu,* Kui Zhao,* “Scalable Ambient Fabrication of High-Performance CsPbI2Br Solar Cells”. Joule, 2019. 3, 2485.

55) Peirui Cheng, Peijun Wang, Zhuo Xu, Xuguang Jia, Qilin Wei, Ningyi Yuan, Jianning Ding, Ruipeng Li, Guangtao Zhao, Yingchun Cheng, Kui Zhao,* and Shengzhong (Frank) Liu*, “Ligand-Size Related Dimensionality Control in Metal Halide Perovskites”. ACS Energy Lett. 2019, 4, 1830.

56) Yalan Zhang, Peijun Wang, Ming-Chun Tang, Dounya Barrit, Weijun Ke, Tao Luo, Yyucheng Liu, Tianqi Niu, Detlef-M. Smilgies, Zhou Yang, Zhike Liu, Shenye Jin, Mercoursi G. Kanatzidis,* Aram Amassian,* Shengzhong (Frank) Liu,* Kui Zhao,* “Dynamical Transformation of 2D Perovskites with Alternating Cations in the Interlayer Space for High-Performance Photovoltaics”. J. Am. Chem. Soc. 2019, 141, 2684.

57) Dounya Barrit, Peirui Cheng, Ming-Chun Tang, Kai Wang, Hoang Dang, Detlef-M. Smilgies, Shengzhong (Frank) Liu, Thomas D. Anthopoulos,* Kui Zhao,* Aram Amassian,* “Impact of the Solvation State of Lead Iodide on its Two-Step Conversion to MAPbI3: An In Situ Investigation”. Adv. Funct. Mater. 2019. 1807544.

58) Tianqi Niu, Jing Lu, Ming-Chun Tang, Dounya Barrit, Detlef-M. Smilgies, Zhou Yang, Jianbo Li, Yuanyuan Fan, Tao Luo, Iain McCulloch, Aram Amassian,* Shengzhong (Frank) Liu,* Kui Zhao,* “High performance ambient-air-stable FAPbI3 perovskite solar cells with molecule-passivated Ruddlesden-Popper/3D heterostructured film”. Energy Environ. Sci. 2018, 11, 3358.

59) Yucheng Liu, Yunxia Zhang, Zhou Yang, Haochen Ye, Jiangshan Feng, Zhuo Xu, Xu Zhang, Rahim Munir, Jianbo Li, Qingxian Li, Mingxi Hu, Liming Meng, Kang Wang, Detlef-M. Smilgies, Aram Amassian, Kui Zhao,* Shengzhong (Frank) Liu,* “Multi-Inch Single-Crystalline Perovskite Membrane for High-Detectivity Flexible Photosensors”. Nat. Commun. 2018, 9, 5302.

60) Peirui Cheng, Zhuo Xu, Jianbo Li, Yucheng Liu, Yuanyuan Fan, Liyang Yu, Detlef-M. Smilgies, Christian Müller, Kui Zhao,* Shengzhong (Frank) Liu,* “Highly Efficient Ruddlesden–Popper Halide Perovskite PA2MA4Pb5I16 Solar Cells”, ACS Energy Lett. 2018, 3, 1975.

61) Yucheng. Liu, Yunxia Zhang, Zhou Yang, Jiangshan Feng, Qinxian Li, Minxi Hu, Xu Zhang, Ming Liu, Kui Zhao,* Shengzhong (Frank) Liu,* “Low Temperature Gradient Crystallization for Multi-Inch High-Quality Perovskite Single-Crystals”. Materials Today 2019, 22, 67.

62) Jianbo Li, Rahim Munir, Yuanyuan Fan, Tianqi Niu, Yucheng Liu, Yufei Zhong, Zhou Yang, Bin Liu, Jie Sun, Detlef-M. Smilgies, Aram Amassian,* Kui Zhao*, Shengzhong (Frank) Liu,* “Phase transition control for high-performance blade-coated perovskite solar cells”, Joule 2018, 2, 1313.

63) Y. Zhong, R. Munir, J. Li, M.-C. Tang, M. Niazi, K. Zhao*, A. Amassian*, “Blade-Coated Perovskite Solar Cells with Efficiency >17%: An In Situ Investigation”. ACS Energy Lett. 2018, 3, 1078.

64) Xu Zhang, Rahim Munir, Zhuo Xu, Yucheng Liu, Hsinhan Tsai, Wanyi Nie, Jianbo Li, Tianqi Niu, Detlef-M. Smilgies, Mercouri G. Kanatzidis, Adtya D. Mohite, Kui Zhao,* Aram Amassian,* Shegnzhong (Frank) Liu,* “Phase Transition Control for High Performance Ruddlesden–Popper Perovskite Solar Cells”. Adv. Mater. 2018, 30, 1707166.

65) T. Niu, J. Lu, R. Munir, J. Li, D. Barrit, X. Zhang, H. Hu, Z. Yang, A. Amassian,* K. Zhao,* S. (Frank) Liu,* “Stable high performance perovskite solar cells via grain boundary passivation”, Adv. Mater. 2018, 30, 1706576.

66) X. Zhang, X. Ren, B. Liu, X. Zhu, D. Yang, J. Li, Y. Liu, D.-M. Smilgies, R. Li, Z. Yang, T. Niu, X. Wang, K. Zhao,* S. (Frank) Liu,* “Stable High Performance Two-Dimensional Perovskite Solar Cells via Cesium Doping”. Energy Environ. Sci. 2017, 10, 2095.



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